I feel like this deserve a thread of its own. So I will start. Please feel free to build on the list or change it (explain why you change it though).

Mobile Suit Gundam

Char Aznable: ENTP
Gihren Zabi: ENTJ
Amuro Ray: ISTP/ISFP
Bright Noa: ESTJ

Gundam Seed

Kira Yamato: INFJ
Lacus Cline: ENFJ
Athrun Zala: ENTP/INFP/ISTP (he seemed to have alot of Fi)
Cagalli: INFP
Dearka Elsman: ESTP
Rau Le Crueset: INTJ
Patrick Zala: ENTX